Tubular carbon molecular sieve (CMS) membranes have been recognized as a potential module for commercial application due to its high mechanical strength and large surface area. However, the carbon layer uniformity was restricted by substrate texture and dope fluidity when the dip-coating method was used. This study evaluated the influence of various parameters of dip-coating with an integrated vacuum-assisted system, including solvent vaporization rates, vertical immersion/withdrawal velocity, vacuum degree, dope composition, coating cycles on the microstructure, and gas separation performance of CMS membranes. Using vacuum assistance and a low-vaporization solvent minimized the influence of viscosity and gravity on dope fluidity as a result of fast phase inversion. The as-prepared tubular CMS membranes showed enhanced perm-selectivity according to a H-2/N(2)gas selectivity of 8.8, a CO2/N(2)gas selectivity of 6.7, a H(2)permeability of 464 barrer, and a CO(2)permeability of 356 barrer.